Highly resolved global distribution of tropospheric NO2 using GOME narrow swath mode data

نویسنده

  • S. Beirle
چکیده

The Global Ozone Monitoring Experiment (GOME) allows the retrieval of tropospheric vertical column densities (VCDs) of NO2 on a global scale. Regions with enhanced industrial activity can clearly be detected, but the standard spatial resolution of the GOME ground pixels (320×40 km2) is insufficient to resolve regional trace gas distributions or individual cities. Every 10 days within the nominal GOME operation, measurements are executed in the so called narrow swath mode with a much better spatial resolution (80×40 km2). We use this data (1997–2001) to construct a detailed picture of the mean global tropospheric NO2 distribution. Since – due to the narrow swath – the global coverage of the high resolution observations is rather poor, it has proved to be essential to deseasonalize the single narrow swath mode observations to retrieve adequate mean maps. This is done by using the GOME backscan information. The retrieved high resolution map illustrates the shortcomings of the standard size GOME pixels and reveals an unprecedented wealth of details in the global distribution of tropospheric NO2. Localised spots of enhanced NO2 VCD can be directly associated to cities, heavy industry centers and even large power plants. Thus our result helps to check emission inventories. The small spatial extent of NO2 “hot spots” allows us to estimate an upper limit of the mean lifetime of boundary layer NOx of 17 h on a global scale. The long time series of GOME data allows a quantitative comparison of the narrow swath mode data to the nominal resolution. Thus we can analyse the dependency of NO2 VCDs on pixel size. This is important for comparing GOME data to results of new satellite instruments like SCIAMACHY (launched March 2002 on ENVISAT), OMI (launched July 2004 on AURA) or GOME II (to be launched 2005) with an improved spatial resolution. Correspondence to: S. Beirle ([email protected])

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Highly resolved global distribution of tropospheric NO2

The Global Ozone Monitoring Experiment (GOME, since 1995) allows the retrieval of global total column densities of atmospheric trace gases, including NO 2. Tropospheric vertical column densities (VCDs) are derived by estimating the stratospheric fraction from measurements over the remote ocean. Mean maps of tropospheric NO 2 VCDs 5 derived from GOME clearly allow to detect regions with enhanced...

متن کامل

Monitoring Nitrogen Oxides with Satellite Instruments: High Resolution Maps from Gome Narrow Swath Mode and Sciamachy

The Global Ozone Monitoring Experiment (GOME) allows to retrieve tropospheric vertical column densities (TVCDs) of NO2. Mean maps of the global distribution of NO2 TVCDs reveal a clear fingerprint of anthropogenic sources due to fossil fuel combustion. However, GOME data suffer from the rather large footprint size of 320 km east-west, leading to a smearing out of the NO2 peaks in the retrieved ...

متن کامل

Tropospheric Oh Primary Production from Ers-2 Data

In order to calculate the OH primary production rate from satellite measurements, one has to estimate the following quantities: profile of the photodissociation rate of ozone to O(D), tropospheric ozone profile and tropospheric water vapour profile. The estimation of tropospheric OH primary production rate from ERS-2 data is demonstrated. The tropospheric ozone profiles retrieved at the Rutherf...

متن کامل

Tropospheric NO2 columns: a comparison between model and retrieved data from GOME measurements

Tropospheric NO2 plays a variety of significant roles in atmospheric chemistry. In the troposphere it is one of the most significant precursors of photochemical ozone (O3) production and nitric acid (HNO3). In this study tropospheric NO2 columns were calculated by the fully coupled chemistry-climate model ECHAM4.L39(DLR)/CHEM. These have been compared with tropospheric NO2 columns, retrieved us...

متن کامل

A transboundary transport episode of nitrogen dioxide as observed from GOME and its impact in the Alpine region

High tropospheric NO2 amounts are occasionally detected by space-borne spectrometers above cloudy scenes. For monitoring of near-ground air pollution such data are not directly applicable because clouds shield the highly polluted planetary boundary layer (PBL). We present a method based on trajectories which implicitly estimates the additional subcloud NO2 distribution in order to model concent...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 2004